? 能源化学(英文)
ISSN 1003-9953
     
能源化学(英文) 2017, Vol. 26 Issue (1) :63-71    DOI: 10.1016/j.jechem.2016.07.005
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Nitrogen-doped cobalt nanoparticles/nitrogen-doped plate-like ordered mesoporous carbons composites as noble-metal free electrocatalysts for oxygen reduction reaction
Vincent Mirai Bau, Xiangjie Bo, Liping Guo
Faculty of Chemistry, Northeast Normal University, Changchun 130024, Jilin, China
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摘要 In this work, nitrogen-doped cobalt nanoparticles/nitrogen-doped plate-like ordered mesoporous carbons (N/Co/OMCs) were used as noble-metal free electrocatalysts with high catalytic efficiency. Compared with OMCs with long channel length, due to more entrances for catalytic target accessibility and a short pathway for rapid diffusion, the utilization efficiency of cobalt nanoparticles inside the plate-like OMCs with short pore length is well improved, which can take full advantage of porous structure in electrocatalysis and increase the utilization of catalysts. The active sites in N/Co/OMCs for oxygen reduction reaction (ORR) are highly exposed to oxygen molecule, which results in a high activity for ORR. By combination of the catalytic properties of nitrogen dopant, incorporation of Co nanoparticles, and structural properties of OMCs, the N/Co/plate-like OMCs are highly active noble-metal free catalysts for ORR in alkaline solution.
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关键词Ordered mesoporous carbons   Nitrogen doping   Cobalt nanoparticles   Oxygen reduction reaction     
收稿日期: 2016-05-10; 发布日期: 2016-07-27
基金资助:

The authors gratefully acknowledge financial support from the National Natural Science Foundation of China (21405011) and the Science and Technology Development Planning of Jilin Province (20150520014JH).

通讯作者 Xiangjie Bo, Liping Guo     Email: baoxj133@nenu.edu.cn;guolp078@nenu.edu.cn
引用本文:   
.Nitrogen-doped cobalt nanoparticles/nitrogen-doped plate-like ordered mesoporous carbons composites as noble-metal free electrocatalysts for oxygen reduction reaction[J]  能源化学(英文) , 2017,V26(1): 63-71
.Nitrogen-doped cobalt nanoparticles/nitrogen-doped plate-like ordered mesoporous carbons composites as noble-metal free electrocatalysts for oxygen reduction reaction[J]  Journal of Energy Chemistry, 2017,V26(1): 63-71
链接本文:  
http://www.jenergchem.org/CN/10.1016/j.jechem.2016.07.005     或     http://www.jenergchem.org/CN/Y2017/V26/I1/63
 
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